Um, JJ, I think you have a bunch of songs on that list that shouldn't be. Here on Corfid, there's a UK concert program with the list of songs he might sing, so I would say it's a safe bet he did all of them at one time or another:
http://www.corfid.com/gl/frank.htm
I have another UK program at home that I can peruse this summer. But, bottom line, I suspect that he did most of the UA stuff in the 60s, because they were all the songs he had! Plus, his arrangements were simple, and most songs could be done solo.